cantera/src/kinetics/importKinetics.cpp

784 lines
27 KiB
C++

/**
* @file importKinetics.cpp
* Declarations of global routines for the importing
* of kinetics data from XML files (see \ref inputfiles).
*
* This file contains routines which are global routines, i.e.,
* not part of any object. These routine take as input, ctml
* pointers to data, and pointers to %Cantera objects. The purpose
* of these routines is to initialize the %Cantera objects with data
* from the ctml tree structures.
*/
// Copyright 2002 California Institute of Technology
#include "cantera/kinetics/importKinetics.h"
#include "cantera/thermo/ThermoFactory.h"
#include "cantera/kinetics/ReactionData.h"
#include "cantera/kinetics/Reaction.h"
#include "cantera/base/stringUtils.h"
#include "cantera/base/ctml.h"
#include <cstring>
using namespace ctml;
using namespace std;
namespace Cantera
{
ReactionRules::ReactionRules() :
skipUndeclaredSpecies(false),
skipUndeclaredThirdBodies(false),
allowNegativeA(false)
{
}
void checkRxnElementBalance(Kinetics& kin,
const ReactionData& rdata, doublereal errorTolerance)
{
warn_deprecated("checkRxnElementBalance", "Now handled by "
"Kinetics::checkReactionBalance. To be removed after Cantera 2.2.");
doublereal kstoich;
map<string, double> bal, balr, balp;
bal.clear();
balp.clear();
balr.clear();
size_t np = rdata.products.size();
// iterate over the products
for (size_t index = 0; index < np; index++) {
size_t kp = rdata.products[index]; // index of the product in 'kin'
size_t n = kin.speciesPhaseIndex(kp); // phase this product belongs to
size_t klocal = kp - kin.kineticsSpeciesIndex(0,n); // index within this phase
kstoich = rdata.pstoich[index]; // product stoichiometric coeff
const ThermoPhase& ph = kin.speciesPhase(kp);
for (size_t m = 0; m < ph.nElements(); m++) {
bal[ph.elementName(m)] += kstoich*ph.nAtoms(klocal,m);
balp[ph.elementName(m)] += kstoich*ph.nAtoms(klocal,m);
}
}
for (size_t index = 0; index < rdata.reactants.size(); index++) {
size_t kr = rdata.reactants[index];
size_t n = kin.speciesPhaseIndex(kr);
size_t klocal = kr - kin.kineticsSpeciesIndex(0,n);
kstoich = rdata.rstoich[index];
const ThermoPhase& ph = kin.speciesPhase(kr);
for (size_t m = 0; m < ph.nElements(); m++) {
bal[ph.elementName(m)] -= kstoich*ph.nAtoms(klocal,m);
balr[ph.elementName(m)] += kstoich*ph.nAtoms(klocal,m);
}
}
map<string, double>::iterator b = bal.begin();
string msg = "\n\tElement Reactants Products";
bool ok = true;
doublereal err, elemsum;
for (; b != bal.end(); ++b) {
elemsum = fabs(balr[b->first]) + fabs(balp[b->first]);
if (elemsum > 0.0) {
err = fabs(b->second/elemsum);
if (err > errorTolerance) {
ok = false;
msg += "\n\t"+b->first+" "+ fp2str(balr[b->first])
+" "+ fp2str(balp[b->first]);
}
}
}
if (!ok) {
msg = "The following reaction is unbalanced:\n\t"
+ rdata.equation + "\n" + msg + "\n";
throw CanteraError("checkRxnElementBalance",msg);
}
}
bool getReagents(const XML_Node& rxn, Kinetics& kin, int rp,
std::string default_phase, std::vector<size_t>& spnum,
vector_fp& stoich, vector_fp& order,
const ReactionRules& rules)
{
warn_deprecated("getReagents", "Now handled through newReaction() and its "
"support functions. To be removed after Cantera 2.2.");
string rptype;
/*
* The id of reactants and products are kept in child elements
* of reaction, named "reactants" and "products". We search
* the xml tree for these children based on the value of rp,
* and store the xml element pointer here.
*/
if (rp == 1) {
rptype = "reactants";
} else {
rptype = "products";
}
const XML_Node& rg = rxn.child(rptype);
/*
* The species and stoichiometric coefficient for the species
* are stored as a colon separated pair. Get all of these
* pairs in the reactions/products object.
*/
std::vector<string> key, val;
ctml::getPairs(rg, key, val);
/*
* Loop over each of the pairs and process them
*/
doublereal ord, stch;
string ph, spName;
map<string, size_t> speciesMap;
for (size_t n = 0; n < key.size(); n++) {
spName = key[n]; // sp is the string name for species
ph = "";
/*
* Search for the species in the kinetics object using the
* member function kineticsSpeciesIndex(). We will search
* for the species in all phases defined in the kinetics operator.
*/
size_t isp = kin.kineticsSpeciesIndex(spName);
if (isp == npos) {
if (rules.skipUndeclaredSpecies) {
return false;
} else {
throw CanteraError("getReagents",
"Undeclared reactant or product species " + spName);
return false;
}
}
/*
* For each reagent, we store the the species number, isp
* the stoichiometric coefficient, val[n], and the order
* species in the reaction rate expression. We assume mass
* action kinetics here, but will modify this below for
* specified species.
*/
spnum.push_back(isp);
stch = fpValue(val[n]);
stoich.push_back(stch);
ord = doublereal(stch);
order.push_back(ord);
/*
* Needed to process reaction orders below.
*/
speciesMap[spName] = order.size();
}
/*
* Check to see if reaction orders have been specified.
*/
if (rp == 1 && rxn.hasChild("order")) {
std::vector<XML_Node*> ord = rxn.getChildren("order");
doublereal forder;
for (size_t nn = 0; nn < ord.size(); nn++) {
const XML_Node& oo = *ord[nn];
string sp = oo["species"];
size_t loc = speciesMap[sp];
if (loc == 0)
throw CanteraError("getReagents",
"reaction order specified for non-reactant: "
+sp);
forder = oo.fp_value();
if (forder < 0.0) {
throw CanteraError("getReagents",
"reaction order must be non-negative");
}
// replace the stoichiometric coefficient
// stored above in 'order' with the specified
// reaction order
order[loc-1] = forder;
}
}
return true;
}
/**
* getArrhenius() parses the xml element called Arrhenius.
* The Arrhenius expression is
* \f[ k = A T^(b) exp (-E_a / RT). \f]
* @deprecated to be removed after Cantera 2.2.
*/
static void getArrhenius(const XML_Node& node, int& labeled,
doublereal& A, doublereal& b, doublereal& E)
{
if (node["name"] == "k0") {
labeled = -1;
} else if (node["name"] == "kHigh") {
labeled = 1;
} else {
labeled = 0;
}
/*
* We parse the children for the A, b, and E components.
*/
A = getFloat(node, "A", "toSI");
b = getFloat(node, "b");
E = getFloat(node, "E", "actEnergy");
E /= GasConstant;
}
/**
* getStick() processes the XML element called Stick that specifies
* the sticking coefficient reaction. This routine will
* translate the sticking coefficient value into a "normal"
* rate constant for the surface reaction.
*
* Output
* -----------
* Output is the normal Arrhenius expressions for a surface
* reaction rate constant.
*
* A - units such that rate of rxn has kmol/m^2/s when
* A is multiplied by activity concentrations of
* reactants in the normal manner.
* n - unitless
* E - Units 1/Kelvin
* @deprecated to be removed after Cantera 2.2.
*/
static void getStick(const XML_Node& node, Kinetics& kin,
ReactionData& r, doublereal& A, doublereal& b, doublereal& E)
{
size_t nr = r.reactants.size();
size_t k, klocal, not_surf = 0;
size_t np = 0;
doublereal f = 1.0;
doublereal order;
/*
* species is the name of the special reactant whose surface
* flux rate will be calculated.
* isp = species # in the local phase
* ispKinetics = species # in the kinetics object
* ispPhaseIndex = phase # of the special species
*/
string spname = node["species"];
ThermoPhase& th = kin.speciesPhase(spname);
size_t isp = th.speciesIndex(spname);
size_t ispKinetics = kin.kineticsSpeciesIndex(spname);
size_t ispPhaseIndex = kin.speciesPhaseIndex(ispKinetics);
doublereal ispMW = th.molecularWeights()[isp];
doublereal sc;
// loop over the reactants
for (size_t n = 0; n < nr; n++) {
k = r.reactants[n];
order = r.rorder[n]; // stoich coeff
// get the phase species k belongs to
np = kin.speciesPhaseIndex(k);
const ThermoPhase& p = kin.thermo(np);
// get the local index of species k in this phase
klocal = p.speciesIndex(kin.kineticsSpeciesName(k));
// if it is a surface species, divide f by the standard
// concentration for this species, in order to convert
// from concentration units used in the law of mass action
// to coverages used in the sticking probability expression
if (p.eosType() == cSurf || p.eosType() == cEdge) {
sc = p.standardConcentration(klocal);
f /= pow(sc, order);
}
// Otherwise:
else {
// We only allow one species to be in the phase containing the
// special sticking coefficient species.
if (ispPhaseIndex == np) {
not_surf++;
}
// Other bulk phase species on the other side of ther interface are
// treated like surface species.
else {
sc = p.standardConcentration(klocal);
f /= pow(sc, order);
}
}
}
if (not_surf != 1) {
throw CanteraError("getStick",
"reaction probabilities can only be used in "
"reactions with exactly 1 gas/liquid species.");
}
doublereal cbar = sqrt(8.0*GasConstant/(Pi*ispMW));
A = 0.25 * getFloat(node, "A", "toSI") * cbar * f;
b = getFloat(node, "b") + 0.5;
E = getFloat(node, "E", "actEnergy");
E /= GasConstant;
}
//! Read the XML data concerning the coverage dependence of an interfacial reaction
/*!
* @param node XML node with name reaction containing the reaction information
* @param surfphase Surface phase
* @param rdata Reaction data for the reaction.
*
* Example:
* @verbatim
<coverage species="CH3*">
<a> 1.0E-5 </a>
<m> 0.0 </m>
<actEnergy> 0.0 </actEnergy>
</coverage>
@endverbatim
* @deprecated to be removed after Cantera 2.2.
*/
static void getCoverageDependence(const XML_Node& node,
thermo_t& surfphase, ReactionData& rdata)
{
vector<XML_Node*> cov = node.getChildren("coverage");
size_t k, nc = cov.size();
doublereal e;
string spname;
if (nc > 0) {
for (size_t n = 0; n < nc; n++) {
const XML_Node& cnode = *cov[n];
spname = cnode["species"];
k = surfphase.speciesIndex(spname);
rdata.cov.push_back(doublereal(k));
rdata.cov.push_back(getFloat(cnode, "a"));
rdata.cov.push_back(getFloat(cnode, "m"));
e = getFloat(cnode, "e", "actEnergy");
rdata.cov.push_back(e/GasConstant);
}
}
}
//! Get falloff parameters for a reaction.
/*!
* This routine reads the falloff XML node and extracts parameters into a
* vector of doubles
*
* @verbatim
<falloff type="Troe"> 0.5 73.2 5000. 9999. </falloff>
@endverbatim
* @deprecated to be removed after Cantera 2.2.
*/
static void getFalloff(const XML_Node& f, ReactionData& rdata)
{
string type = f["type"];
vector<string> p;
getStringArray(f,p);
vector_fp c;
size_t np = p.size();
for (size_t n = 0; n < np; n++) {
c.push_back(fpValue(p[n]));
}
if (type == "Troe") {
if (np == 3 || np == 4) {
rdata.falloffType = TROE_FALLOFF;
} else {
throw CanteraError("getFalloff()", "Troe parameterization is specified by number of parameters, "
+ int2str(np) + ", is not equal to 3 or 4");
}
} else if (type == "SRI") {
if (np == 3 || np == 5) {
rdata.falloffType = SRI_FALLOFF;
} else {
throw CanteraError("getFalloff()", "SRI parameterization is specified by number of parameters, "
+ int2str(np) + ", is not equal to 3 or 5");
}
}
rdata.falloffParameters = c;
}
/**
* Get the enhanced collision efficiencies. It is assumed that the
* reaction mechanism is homogeneous, so that all species belong
* to phase(0) of 'kin'.
* @deprecated to be removed after Cantera 2.2.
*/
static void getEfficiencies(const XML_Node& eff, Kinetics& kin,
ReactionData& rdata, const ReactionRules& rules)
{
// set the default collision efficiency
rdata.default_3b_eff = fpValue(eff["default"]);
vector<string> key, val;
ctml::getPairs(eff, key, val);
string nm;
string phse = kin.thermo(0).id();
for (size_t n = 0; n < key.size(); n++) {
nm = key[n];
size_t k = kin.kineticsSpeciesIndex(nm, phse);
if (k != npos) {
rdata.thirdBodyEfficiencies[k] = fpValue(val[n]);
} else if (!rules.skipUndeclaredThirdBodies) {
throw CanteraError("getEfficiencies", "Encountered third-body "
"efficiency for undefined species \"" + nm + "\"\n"
"while adding reaction " + int2str(rdata.number+1) + ".");
}
}
}
void getRateCoefficient(const XML_Node& kf, Kinetics& kin,
ReactionData& rdata, const ReactionRules& rules)
{
warn_deprecated("getRateCoefficent", "Now handled through newReaction() "
"and its support functions. To be removed after Cantera 2.2.");
if (rdata.reactionType == PLOG_RXN) {
rdata.rateCoeffType = PLOG_REACTION_RATECOEFF_TYPE;
for (size_t m = 0; m < kf.nChildren(); m++) {
const XML_Node& node = kf.child(m);
double p = getFloat(node, "P", "toSI");
vector_fp& rate = rdata.plogParameters.insert(
std::make_pair(p, vector_fp()))->second;
rate.resize(3);
rate[0] = getFloat(node, "A", "toSI");
rate[1] = getFloat(node, "b");
rate[2] = getFloat(node, "E", "actEnergy") / GasConstant;
}
} else if (rdata.reactionType == CHEBYSHEV_RXN) {
rdata.rateCoeffType = CHEBYSHEV_REACTION_RATECOEFF_TYPE;
rdata.chebTmin = getFloat(kf, "Tmin", "toSI");
rdata.chebTmax = getFloat(kf, "Tmax", "toSI");
rdata.chebPmin = getFloat(kf, "Pmin", "toSI");
rdata.chebPmax = getFloat(kf, "Pmax", "toSI");
const XML_Node& coeffs = kf.child("floatArray");
rdata.chebDegreeP = atoi(coeffs["degreeP"].c_str());
rdata.chebDegreeT = atoi(coeffs["degreeT"].c_str());
getFloatArray(kf, rdata.chebCoeffs, false);
} else {
string type = kf.attrib("type");
if (type == "") {
type = "Arrhenius";
rdata.rateCoeffType = ARRHENIUS_REACTION_RATECOEFF_TYPE;
}
if (type == "ExchangeCurrentDensity") {
rdata.rateCoeffType = EXCHANGE_CURRENT_REACTION_RATECOEFF_TYPE;
} else if (type == "Arrhenius") {
} else {
throw CanteraError("getRateCoefficient", "Unknown type: " + type);
}
vector_fp c_alt(3,0.0), c_base(3,0.0);
for (size_t m = 0; m < kf.nChildren(); m++) {
const XML_Node& c = kf.child(m);
string nm = c.name();
int labeled=0;
if (nm == "Arrhenius") {
vector_fp coeff(3);
if (c["type"] == "stick") {
getStick(c, kin, rdata, coeff[0], coeff[1], coeff[2]);
c_base = coeff;
} else {
getArrhenius(c, labeled, coeff[0], coeff[1], coeff[2]);
if (labeled == 0 || rdata.reactionType == THREE_BODY_RXN
|| rdata.reactionType == ELEMENTARY_RXN) {
c_base = coeff;
} else {
c_alt = coeff;
}
}
if (rdata.reactionType == SURFACE_RXN || rdata.reactionType == EDGE_RXN) {
getCoverageDependence(c,
kin.thermo(kin.surfacePhaseIndex()), rdata);
}
if (coeff[0] < 0.0 && !rules.allowNegativeA) {
throw CanteraError("getRateCoefficient",
"negative A coefficient for reaction "+int2str(rdata.number));
}
} else if (nm == "Arrhenius_ExchangeCurrentDensity") {
vector_fp coeff(3);
getArrhenius(c, labeled, coeff[0], coeff[1], coeff[2]);
c_base = coeff;
rdata.rateCoeffType = EXCHANGE_CURRENT_REACTION_RATECOEFF_TYPE;
} else if (nm == "falloff") {
getFalloff(c, rdata);
} else if (nm == "efficiencies") {
getEfficiencies(c, kin, rdata, rules);
} else if (nm == "electrochem") {
rdata.beta = fpValue(c["beta"]);
}
}
/*
* Store the coefficients in the ReactionData object for return
* from this function.
*/
if (rdata.reactionType == FALLOFF_RXN) {
rdata.rateCoeffParameters = c_base;
rdata.auxRateCoeffParameters = c_alt;
} else if (rdata.reactionType == CHEMACT_RXN) {
rdata.rateCoeffParameters = c_alt;
rdata.auxRateCoeffParameters = c_base;
} else {
rdata.rateCoeffParameters = c_base;
}
}
}
doublereal isDuplicateReaction(std::map<int, doublereal>& r1,
std::map<int, doublereal>& r2)
{
warn_deprecated("isDuplicateReaction", "Now handled by "
"Kinetics::checkDuplicateStoich. To be removed after Cantera 2.2.");
map<int, doublereal>::const_iterator b = r1.begin(), e = r1.end();
int k1 = b->first;
// check for duplicate written in the same direction
doublereal ratio = 0.0;
if (r1[k1] && r2[k1]) {
ratio = r2[k1]/r1[k1];
++b;
bool different = false;
for (; b != e; ++b) {
k1 = b->first;
if (!r1[k1] || !r2[k1] || fabs(r2[k1]/r1[k1] - ratio) > 1.e-8) {
different = true;
break;
}
}
if (!different) {
return ratio;
}
}
// check for duplicate written in the reverse direction
b = r1.begin();
k1 = b->first;
if (r1[k1] == 0.0 || r2[-k1] == 0.0) {
return 0.0;
}
ratio = r2[-k1]/r1[k1];
++b;
for (; b != e; ++b) {
k1 = b->first;
if (!r1[k1] || !r2[-k1] || fabs(r2[-k1]/r1[k1] - ratio) > 1.e-8) {
return 0.0;
}
}
return ratio;
}
bool installReactionArrays(const XML_Node& p, Kinetics& kin,
std::string default_phase, bool check_for_duplicates)
{
int itot = 0;
/*
* Search the children of the phase element for the
* xml element named reactionArray. If we can't find it,
* then return signaling having not found any reactions.
* Apparently, we allow multiple reactionArray elements here
* Each one will be processed sequentially, with the
* end result being purely additive.
*/
vector<XML_Node*> rarrays = p.getChildren("reactionArray");
if (rarrays.empty()) {
kin.finalize();
return false;
}
for (size_t n = 0; n < rarrays.size(); n++) {
/*
* Go get a reference to the current xml element,
* reactionArray. We will process this element now.
*/
const XML_Node& rxns = *rarrays[n];
/*
* The reactionArray element has an attribute called,
* datasrc. The value of the attribute is the xml
* element comprising the top of the
* tree of reactions for the phase.
* Find this datasrc element starting with the root
* of the current xml node.
*/
const XML_Node* rdata = get_XML_Node(rxns["datasrc"], &rxns.root());
/*
* If the reactionArray element has a child element named "skip", and
* if the attribute of skip called "species" has a value of "undeclared",
* we will set rxnrule.skipUndeclaredSpecies to 'true'. rxnrule is
* passed to the routine that parses each individual reaction so that
* the parser will skip all reactions containing an undefined species
* without throwing an error.
*
* Similarly, an attribute named "third_bodies" with the value of
* "undeclared" will skip undeclared third body efficiencies (while
* retaining the reaction and any other efficiencies).
*/
if (rxns.hasChild("skip")) {
const XML_Node& sk = rxns.child("skip");
if (sk["species"] == "undeclared") {
kin.skipUndeclaredSpecies(true);
}
if (sk["third_bodies"] == "undeclared") {
kin.skipUndeclaredThirdBodies(true);
}
}
/*
* Search for child elements called include. We only include
* a reaction if it's tagged by one of the include fields.
* Or, we include all reactions if there are no include fields.
*/
vector<XML_Node*> incl = rxns.getChildren("include");
vector<XML_Node*> allrxns = rdata->getChildren("reaction");
// if no 'include' directive, then include all reactions
if (incl.empty()) {
for (size_t i = 0; i < allrxns.size(); i++) {
kin.addReaction(newReaction(*allrxns[i]));
++itot;
}
} else {
for (size_t nii = 0; nii < incl.size(); nii++) {
const XML_Node& ii = *incl[nii];
string imin = ii["min"];
string imax = ii["max"];
string::size_type iwild = string::npos;
if (imax == imin) {
iwild = imin.find("*");
if (iwild != string::npos) {
imin = imin.substr(0,iwild);
imax = imin;
}
}
for (size_t i = 0; i < allrxns.size(); i++) {
const XML_Node* r = allrxns[i];
string rxid;
if (r) {
rxid = r->attrib("id");
if (iwild != string::npos) {
rxid = rxid.substr(0,iwild);
}
/*
* To decide whether the reaction is included or not
* we do a lexical min max and operation. This
* sometimes has surprising results.
*/
if ((rxid >= imin) && (rxid <= imax)) {
kin.addReaction(newReaction(*r));
++itot;
}
}
}
}
}
}
if (check_for_duplicates) {
kin.checkDuplicates();
}
/*
* Finalize the installation of the kinetics, now that we know
* the true number of reactions in the mechanism, itot.
*/
kin.finalize();
return true;
}
bool importKinetics(const XML_Node& phase, std::vector<ThermoPhase*> th,
Kinetics* k)
{
if (k == 0) {
return false;
}
// This phase will be the owning phase for the kinetics operator
// For interfaces, it is the surface phase between two volumes.
// For homogeneous kinetics, it's the current volumetric phase.
string owning_phase = phase["id"];
bool check_for_duplicates = false;
if (phase.parent()) {
if (phase.parent()->hasChild("validate")) {
const XML_Node& d = phase.parent()->child("validate");
if (d["reactions"] == "yes") {
check_for_duplicates = true;
}
}
}
// if other phases are involved in the reaction mechanism,
// they must be listed in a 'phaseArray' child
// element. Homogeneous mechanisms do not need to include a
// phaseArray element.
vector<string> phase_ids;
if (phase.hasChild("phaseArray")) {
const XML_Node& pa = phase.child("phaseArray");
getStringArray(pa, phase_ids);
}
phase_ids.push_back(owning_phase);
int np = static_cast<int>(phase_ids.size());
int nt = static_cast<int>(th.size());
// for each referenced phase, attempt to find its id among those
// phases specified.
bool phase_ok;
string phase_id;
string msg = "";
for (int n = 0; n < np; n++) {
phase_id = phase_ids[n];
phase_ok = false;
// loop over the supplied 'ThermoPhase' objects representing
// phases, to find an object with the same id.
for (int m = 0; m < nt; m++) {
if (th[m]->id() == phase_id) {
phase_ok = true;
// if no phase with this id has been added to
//the kinetics manager yet, then add this one
if (k->phaseIndex(phase_id) == npos) {
k->addPhase(*th[m]);
}
}
msg += " "+th[m]->id();
}
if (!phase_ok) {
throw CanteraError("importKinetics",
"phase "+phase_id+" not found. Supplied phases are:"+msg);
}
}
// allocates arrays, etc. Must be called after the phases have
// been added to 'kin', so that the number of species in each
// phase is known.
k->init();
// Install the reactions.
return installReactionArrays(phase, *k, owning_phase, check_for_duplicates);
}
bool buildSolutionFromXML(XML_Node& root, const std::string& id,
const std::string& nm, ThermoPhase* th, Kinetics* kin)
{
XML_Node* x;
x = get_XML_NameID(nm, string("#")+id, &root);
if (!x) {
return false;
}
/*
* Fill in the ThermoPhase object by querying the
* const XML_Node tree located at x.
*/
importPhase(*x, th);
/*
* Create a vector of ThermoPhase pointers of length 1
* having the current th ThermoPhase as the entry.
*/
std::vector<ThermoPhase*> phases(1);
phases[0] = th;
/*
* Fill in the kinetics object k, by querying the
* const XML_Node tree located by x. The source terms and
* eventually the source term vector will be constructed
* from the list of ThermoPhases in the vector, phases.
*/
importKinetics(*x, phases, kin);
return true;
}
}